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Abstract The magnetic ground state of the pyrochlore Yb 2 GaSbO 7 has not been established. The persistent spin fluctuations observed by muon spin-relaxation measurements at low temperatures have not been adequately explained for this material using existing theories for quantum magnetism. Here we report on the synthesis and characterisation of Yb 2 GaSbO 7 to revisit the nature of the magnetic ground state. Through DC and AC magnetic susceptibility, heat capacity, and neutron scattering experiments, we observe evidence for a dynamical ground state that makes Yb 2 GaSbO 7 a promising candidate for disorder-induced spin-liquid or spin-singlet behaviour. This state is quite fragile, being tuned to a splayed ferromagnet in a modest magnetic field μ 0 H c ~ 1.5 T.more » « less
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Graves, W. S. ; Bessuille, J. ; Brown, P. ; Carbajo, S. ; Dolgashev, V. ; Hong, K.-H. ; Ihloff, E. ; Khaykovich, B. ; Lin, H. ; Murari, K. ; et al ( , Physical Review Special Topics - Accelerators and Beams)